Chemistry

Advances in Chemical Physics [Vol 15] by Stuart A Rice; I Prigogine

By Stuart A Rice; I Prigogine

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It depends only on the distribution of the units over the physical states. (b) The elimination of correlations means also the elimination of virtual states. In the initial representation the evolution of the situation may be described graphically as in Figure 6. Particles are colliding and interacting” at the same time. N o clear distinction between a real collision “ ” “ W Fig. 6 “ ” 30 I. PRIGOGINE process between particles a and b and a “virtual ” process leading to the interaction between a and c can be made.

Shuler Copyright © 1969 by John Wiley & Sons. Inc. RELAXED MOTION IN IRREVERSIBLE MOLECULAR STATISTICS B. 0. KOOPMAN Department of Mathematics, Columbia University, New York, New York CONTENTS I. The Basic Enigma . . . . . . . . . . . . . . IV. The Information Content of Probability Statements . V. Heuristic Introduction to Relaxed Motion . . VI. Plan of Explicit Calculation . . . . 11. The Basic Macroscopic Functions 111. The Boundary Forces . . VII. Solution in a Simplified Case: “Vestiginal VIJI.

These expressions were derived until recently in the weakly coupled limit, or for dilute gases. 14 It appears as a natural generalization of Landau’s theory of quasi-particles in the case when dissipation can no longer be neglected. The most interesting feature is that equilibrium and nonequilibrium properties appear linked. The very definition of the strongly coupled anharmonic phonons depends on their lifetime. l2, l 3 In particle physics it leads to a clear separation of dressing and dynamic effects and permits, therefore, a unified treatment of both stable and unstable states.

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